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2024 | OriginalPaper | Buchkapitel

Activity Descriptors for Atomically Precise HER Electrocatalysts

verfasst von : Yasemin Aykut, Ayşe Bayrakçeken Yurtcan

Erschienen in: Atomically Precise Electrocatalysts for Electrochemical Energy Applications

Verlag: Springer Nature Switzerland

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Abstract

In electrochemistry, the hydrogen evolution reaction (HER) ranks among the most significant reactions. HER is the easiest method to produce very pure hydrogen so the development of effective HER catalysts is of great importance. This situation has significantly influenced many researchers in the field of electrochemistry and made it the focus of active studies. In this direction, many catalysts with different structures have been developed for HER over many years. Among the various HER catalysts, atomically precise electrocatalysts (single-atom, dual-atom, and multi-atom) are becoming more popular because of their efficient use of atoms and impressive electrocatalytic performance. Recently, researchers have made significant efforts to synthesize and develop atomically precise HER catalysts with high activity and stability. However, it is critical to descriptor new strategies to improve catalytic activity. Therefore, different descriptors have been developed to describe the correlation between catalyst morphology and activity. In this chapter, we summarized the activity descriptors commonly used in the design of atomically precise HER catalysts and their importance. We also discussed their impact on performance. Finally, strategies developed to identify new descriptors for promising HER catalysts are proposed.

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Literatur
Zurück zum Zitat Bruix A, Rodriguez JA, Ramírez PJ, Senanayake SD, Evans J, Park JB, Stacchiola D, Liu P, Hrbek J, Illas F (2012) A new type of strong metal-support interaction and the production of H2 through the transformation of water on Pt/CeO2(111) and Pt/CeOx/TiO2(110) catalysts. J Am Chem Soc 134:8968–8974CrossRef Bruix A, Rodriguez JA, Ramírez PJ, Senanayake SD, Evans J, Park JB, Stacchiola D, Liu P, Hrbek J, Illas F (2012) A new type of strong metal-support interaction and the production of H2 through the transformation of water on Pt/CeO2(111) and Pt/CeOx/TiO2(110) catalysts. J Am Chem Soc 134:8968–8974CrossRef
Zurück zum Zitat Calle-Vallejo F, Tymoczko J, Colic V, Vu QH, Pohl MD, Morgenstern K, Loffreda D, Sautet P, Schuhmann W, Bandarenka AS (2015) Finding optimal surface sites on heterogeneous catalysts by counting nearest neighbors. Science 350:185–189CrossRef Calle-Vallejo F, Tymoczko J, Colic V, Vu QH, Pohl MD, Morgenstern K, Loffreda D, Sautet P, Schuhmann W, Bandarenka AS (2015) Finding optimal surface sites on heterogeneous catalysts by counting nearest neighbors. Science 350:185–189CrossRef
Zurück zum Zitat Chang Y, Cheng Y, Feng Y, Li K, Jian H, Zhang H (2019) Upshift of the d band center toward the fermi level for promoting silver ion release, bacteria inactivation, and wound healing of alloy silver nanoparticles. ACS Appl Mater Interfaces 11:12224–12231CrossRef Chang Y, Cheng Y, Feng Y, Li K, Jian H, Zhang H (2019) Upshift of the d band center toward the fermi level for promoting silver ion release, bacteria inactivation, and wound healing of alloy silver nanoparticles. ACS Appl Mater Interfaces 11:12224–12231CrossRef
Zurück zum Zitat Chao T, Luo X, Chen W, Jiang B, Ge J, Lin Y, Wu G, Wang X, Hu Y, Zhuang Z, Wu Y, Hong X, Li Y (2017) Atomically dispersed copper-platinum dual sites alloyed with palladium nanorings catalyze the hydrogen evolution reaction. Angew Chem Int Ed 56:16047–16051CrossRef Chao T, Luo X, Chen W, Jiang B, Ge J, Lin Y, Wu G, Wang X, Hu Y, Zhuang Z, Wu Y, Hong X, Li Y (2017) Atomically dispersed copper-platinum dual sites alloyed with palladium nanorings catalyze the hydrogen evolution reaction. Angew Chem Int Ed 56:16047–16051CrossRef
Zurück zum Zitat Chen M, Smart TJ, Wang S, Kou T, Lin D, Ping Y, Li Y (2020) The coupling of experiments with density functional theory in the studies of the electrochemical hydrogen evolution reaction. J Mater Chem A 8:8783–8812CrossRef Chen M, Smart TJ, Wang S, Kou T, Lin D, Ping Y, Li Y (2020) The coupling of experiments with density functional theory in the studies of the electrochemical hydrogen evolution reaction. J Mater Chem A 8:8783–8812CrossRef
Zurück zum Zitat Cheng Q, Hu C, Wang G, Zou Z, Yang H, Dai L (2020) Carbon-defect-driven electroless deposition of Pt atomic clusters for highly efficient hydrogen evolution. J Am Chem Soc 142:5594–5601CrossRef Cheng Q, Hu C, Wang G, Zou Z, Yang H, Dai L (2020) Carbon-defect-driven electroless deposition of Pt atomic clusters for highly efficient hydrogen evolution. J Am Chem Soc 142:5594–5601CrossRef
Zurück zum Zitat Durst J, Siebel A, Simon C, Hasché F, Herranz J, Gasteiger HA (2014) New insights into the electrochemical hydrogen oxidation and evolution reaction mechanism. Energy Environ Sci 7:2255–2260CrossRef Durst J, Siebel A, Simon C, Hasché F, Herranz J, Gasteiger HA (2014) New insights into the electrochemical hydrogen oxidation and evolution reaction mechanism. Energy Environ Sci 7:2255–2260CrossRef
Zurück zum Zitat Elbert K, Hu J, Ma Z, Zhang Y, Chen G, An W, Liu P, Isaacs HS, Adzic RR, Wang JX (2015) Elucidating hydrogen oxidation/evolution kinetics in base and acid by enhanced activities at the optimized Pt shell thickness on the Ru core. ACS Catal 5:6764–6772CrossRef Elbert K, Hu J, Ma Z, Zhang Y, Chen G, An W, Liu P, Isaacs HS, Adzic RR, Wang JX (2015) Elucidating hydrogen oxidation/evolution kinetics in base and acid by enhanced activities at the optimized Pt shell thickness on the Ru core. ACS Catal 5:6764–6772CrossRef
Zurück zum Zitat Fung V, Hu G, Wu Z, Jiang D-E (2020) Descriptors for hydrogen evolution on single atom catalysts in nitrogen-doped graphene. J Phys Chem C. 124:19571–19578 Fung V, Hu G, Wu Z, Jiang D-E (2020) Descriptors for hydrogen evolution on single atom catalysts in nitrogen-doped graphene. J Phys Chem C. 124:19571–19578
Zurück zum Zitat Gao X, Yu G, Zheng L, Zhang C, Li H, Wang T, An P, Liu M, Qiu X, Chen W, Chen W (2019) Strong electron coupling from the sub-nanometer Pd clusters confined in porous ceria nanorods for highly efficient electrochemical hydrogen evolution reaction. ACS Appl Energy Mater 2:966–973CrossRef Gao X, Yu G, Zheng L, Zhang C, Li H, Wang T, An P, Liu M, Qiu X, Chen W, Chen W (2019) Strong electron coupling from the sub-nanometer Pd clusters confined in porous ceria nanorods for highly efficient electrochemical hydrogen evolution reaction. ACS Appl Energy Mater 2:966–973CrossRef
Zurück zum Zitat Ge J, Zhang D, Qin Y, Dou T, Jiang M, Zhang F, Lei X (2021) Dual-metallic single Ru and Ni atoms decoration of MoS2 for high-efficiency hydrogen production. Appl Catal B 298:120557CrossRef Ge J, Zhang D, Qin Y, Dou T, Jiang M, Zhang F, Lei X (2021) Dual-metallic single Ru and Ni atoms decoration of MoS2 for high-efficiency hydrogen production. Appl Catal B 298:120557CrossRef
Zurück zum Zitat Guo J, Shang W, Hu J, Xin C, Cheng X, Wei J, Zhu C, Liu W, Shi Y (2022) Synergistically enhanced single-atom nickel catalysis for alkaline hydrogen evolution reaction. ACS Appl Mater Interfaces 14:29822–29831CrossRef Guo J, Shang W, Hu J, Xin C, Cheng X, Wei J, Zhu C, Liu W, Shi Y (2022) Synergistically enhanced single-atom nickel catalysis for alkaline hydrogen evolution reaction. ACS Appl Mater Interfaces 14:29822–29831CrossRef
Zurück zum Zitat Hammer B, Norskov JK (1995) Why gold is the noblest of all the metals. Nature 376:238–240CrossRef Hammer B, Norskov JK (1995) Why gold is the noblest of all the metals. Nature 376:238–240CrossRef
Zurück zum Zitat Hu C, Song E, Wang M, Chen W, Huang F, Feng Z, Liu J, Wang J (2021) Partial-single-atom, partial-nanoparticle composites enhance water dissociation for hydrogen evolution. Adv Sci 8:2001881CrossRef Hu C, Song E, Wang M, Chen W, Huang F, Feng Z, Liu J, Wang J (2021) Partial-single-atom, partial-nanoparticle composites enhance water dissociation for hydrogen evolution. Adv Sci 8:2001881CrossRef
Zurück zum Zitat Jiang K, Luo M, Liu Z, Peng M, Chen D, Lu Y-R, Chan T-S, de Groot FM, Tan Y (2021) Rational strain engineering of single-atom ruthenium on nanoporous MoS2 for highly efficient hydrogen evolution. Nat Commun 12:1687CrossRef Jiang K, Luo M, Liu Z, Peng M, Chen D, Lu Y-R, Chan T-S, de Groot FM, Tan Y (2021) Rational strain engineering of single-atom ruthenium on nanoporous MoS2 for highly efficient hydrogen evolution. Nat Commun 12:1687CrossRef
Zurück zum Zitat Jiao M, Chen Z, Wang N, Liu L (2023) DFT calculation screened CoCu and CoFe dual-atom catalysts with remarkable hydrogen evolution reaction activity. Appl Catal B 324:122244CrossRef Jiao M, Chen Z, Wang N, Liu L (2023) DFT calculation screened CoCu and CoFe dual-atom catalysts with remarkable hydrogen evolution reaction activity. Appl Catal B 324:122244CrossRef
Zurück zum Zitat Kumar A, Bui VQ, Lee J, Wang L, Jadhav AR, Liu X, Shao X, Liu Y, Yu J, Hwang Y, Bui HTD, Ajmal S, Kim MG, Kim S-G, Park G-S, Kawazoe Y, Lee H (2021) Moving beyond bimetallic-alloy to single-atom dimer atomic-interface for all-pH hydrogen evolution. Nat Commun 12:6766 Kumar A, Bui VQ, Lee J, Wang L, Jadhav AR, Liu X, Shao X, Liu Y, Yu J, Hwang Y, Bui HTD, Ajmal S, Kim MG, Kim S-G, Park G-S, Kawazoe Y, Lee H (2021) Moving beyond bimetallic-alloy to single-atom dimer atomic-interface for all-pH hydrogen evolution. Nat Commun 12:6766
Zurück zum Zitat Liu X, Jiao Y, Zheng Y, Davey K, Qiao S-Z (2019a) A computational study on Pt and Ru dimers supported on graphene for the hydrogen evolution reaction: new insight into the alkaline mechanism. J Mater Chem A 7:3648–3654CrossRef Liu X, Jiao Y, Zheng Y, Davey K, Qiao S-Z (2019a) A computational study on Pt and Ru dimers supported on graphene for the hydrogen evolution reaction: new insight into the alkaline mechanism. J Mater Chem A 7:3648–3654CrossRef
Zurück zum Zitat Liu F, Shi C, Guo X, He Z, Pan L, Huang ZF, Zhang X, Zou JJ (2022a) Rational design of better hydrogen evolution electrocatalysts for water splitting: a review. Adv Sci 9:2200307CrossRef Liu F, Shi C, Guo X, He Z, Pan L, Huang ZF, Zhang X, Zou JJ (2022a) Rational design of better hydrogen evolution electrocatalysts for water splitting: a review. Adv Sci 9:2200307CrossRef
Zurück zum Zitat Liu X, Deng Y, Zheng L, Kesama MR, Tang C, Zhu Y (2022b) Engineering low-coordination single-atom cobalt on graphitic carbon nitride catalyst for hydrogen evolution. ACS Catal 12:5517–5526CrossRef Liu X, Deng Y, Zheng L, Kesama MR, Tang C, Zhu Y (2022b) Engineering low-coordination single-atom cobalt on graphitic carbon nitride catalyst for hydrogen evolution. ACS Catal 12:5517–5526CrossRef
Zurück zum Zitat Liu J, Wang Z, Kou L, Gu Y (2023) Mechanism exploration and catalyst design for hydrogen evolution reaction accelerated by density functional theory simulations. ACS Sustain Chem Eng 11:467–481CrossRef Liu J, Wang Z, Kou L, Gu Y (2023) Mechanism exploration and catalyst design for hydrogen evolution reaction accelerated by density functional theory simulations. ACS Sustain Chem Eng 11:467–481CrossRef
Zurück zum Zitat Liu E, Li J, Jiao L, Doan HTT, Liu Z, Zhao Z, Huang Y, Abraham K, Mukerjee S, Jia Q (2019) Unifying the hydrogen evolution and oxidation reactions kinetics in base by identifying the catalytic roles of hydroxyl-water-cation adducts. J. Am. Chem. Soc. 141:3232–3239 Liu E, Li J, Jiao L, Doan HTT, Liu Z, Zhao Z, Huang Y, Abraham K, Mukerjee S, Jia Q (2019) Unifying the hydrogen evolution and oxidation reactions kinetics in base by identifying the catalytic roles of hydroxyl-water-cation adducts. J. Am. Chem. Soc. 141:3232–3239
Zurück zum Zitat Lu B, Guo L, Wu F, Peng Y, Lu JE, Smart TJ, Wang N, Finfrock YZ, Morris D, Zhang P, Li N, Gao P, Ping Y, Chen S (2019) Ruthenium atomically dispersed in carbon outperforms platinum toward hydrogen evolution in alkaline media. Nat Commun 10:631CrossRef Lu B, Guo L, Wu F, Peng Y, Lu JE, Smart TJ, Wang N, Finfrock YZ, Morris D, Zhang P, Li N, Gao P, Ping Y, Chen S (2019) Ruthenium atomically dispersed in carbon outperforms platinum toward hydrogen evolution in alkaline media. Nat Commun 10:631CrossRef
Zurück zum Zitat Luo Y, Zhang S, Pan H, Xiao S, Guo Z, Tang L, Khan U, Ding B-F, Li M, Cai Z, Zhao Y, Lv W, Feng Q, Zou X, Lin J, Cheng H-M, Liu B (2020) Unsaturated single atoms on monolayer transition metal dichalcogenides for ultrafast hydrogen evolution. ACS Nano 14:767–776CrossRef Luo Y, Zhang S, Pan H, Xiao S, Guo Z, Tang L, Khan U, Ding B-F, Li M, Cai Z, Zhao Y, Lv W, Feng Q, Zou X, Lin J, Cheng H-M, Liu B (2020) Unsaturated single atoms on monolayer transition metal dichalcogenides for ultrafast hydrogen evolution. ACS Nano 14:767–776CrossRef
Zurück zum Zitat Nørskov JK, Holloway S, Lang ND (1984) Microscopic model for the poisoning and promotion of adsorption rates by electronegative and electropositive atoms. Surf Sci 137:65–78CrossRef Nørskov JK, Holloway S, Lang ND (1984) Microscopic model for the poisoning and promotion of adsorption rates by electronegative and electropositive atoms. Surf Sci 137:65–78CrossRef
Zurück zum Zitat Peng W, Feng Y, Yan X, Hou F, Wang L, Liang J (2021) Multiatom catalysts for energy-related electrocatalysis. Adv Sustain Syst 5:2000213CrossRef Peng W, Feng Y, Yan X, Hou F, Wang L, Liang J (2021) Multiatom catalysts for energy-related electrocatalysis. Adv Sustain Syst 5:2000213CrossRef
Zurück zum Zitat Qi L, Gao W, Jiang Q (2020) Effective descriptor for designing high-performance catalysts for the hydrogen evolution reaction. J Phys Chem C 124:23134–23142CrossRef Qi L, Gao W, Jiang Q (2020) Effective descriptor for designing high-performance catalysts for the hydrogen evolution reaction. J Phys Chem C 124:23134–23142CrossRef
Zurück zum Zitat Su P, Pei W, Wang X, Ma Y, Jiang Q, Liang J, Zhou S, Zhao J, Liu J, Lu GQ (2021) Exceptional electrochemical HER performance with enhanced electron transfer between Ru nanoparticles and single atoms dispersed on a carbon substrate. Angew Chem Int Ed 60:16044–16050CrossRef Su P, Pei W, Wang X, Ma Y, Jiang Q, Liang J, Zhou S, Zhao J, Liu J, Lu GQ (2021) Exceptional electrochemical HER performance with enhanced electron transfer between Ru nanoparticles and single atoms dispersed on a carbon substrate. Angew Chem Int Ed 60:16044–16050CrossRef
Zurück zum Zitat Subbaraman R, Tripkovic D, Strmcnik D, Chang K-C, Uchimura M, Paulikas AP, Stamenkovic V, Markovic NM (2011) Enhancing hydrogen evolution activity in water splitting by tailoring Li+–Ni (OH) 2-Pt interfaces. Science 334:1256–1260CrossRef Subbaraman R, Tripkovic D, Strmcnik D, Chang K-C, Uchimura M, Paulikas AP, Stamenkovic V, Markovic NM (2011) Enhancing hydrogen evolution activity in water splitting by tailoring Li+–Ni (OH) 2-Pt interfaces. Science 334:1256–1260CrossRef
Zurück zum Zitat Sun Y, Zang Y, Tian W, Yu X, Qi J, Chen L, Liu X, Qiu H (2022) Plasma-induced large-area N, Pt-doping and phase engineering of MoS2 nanosheets for alkaline hydrogen evolution. Energy Environ Sci 15:1201–1210CrossRef Sun Y, Zang Y, Tian W, Yu X, Qi J, Chen L, Liu X, Qiu H (2022) Plasma-induced large-area N, Pt-doping and phase engineering of MoS2 nanosheets for alkaline hydrogen evolution. Energy Environ Sci 15:1201–1210CrossRef
Zurück zum Zitat Wu Q, Li H, Zhou Y, Lv S, Chen T, Liu S, Li W, Chen Z (2022) Convenient synthesis of a Ru catalyst containing single atoms and nanoparticles on nitrogen-doped carbon with superior hydrogen evolution reaction activity in a wide pH range. Inorg Chem 61:11011–11021CrossRef Wu Q, Li H, Zhou Y, Lv S, Chen T, Liu S, Li W, Chen Z (2022) Convenient synthesis of a Ru catalyst containing single atoms and nanoparticles on nitrogen-doped carbon with superior hydrogen evolution reaction activity in a wide pH range. Inorg Chem 61:11011–11021CrossRef
Zurück zum Zitat Xu H, Cheng D, Cao D, Zeng XC (2018) A universal principle for a rational design of single-atom electrocatalysts. Nat Catal 1:339–348CrossRef Xu H, Cheng D, Cao D, Zeng XC (2018) A universal principle for a rational design of single-atom electrocatalysts. Nat Catal 1:339–348CrossRef
Zurück zum Zitat Xu F, Zhao J, Wang J, Guan T, Li K (2022) Strong coordination ability of sulfur with cobalt for facilitating scale-up synthesis of Co9S8 encapsulated S, N co-doped carbon as a trifunctional electrocatalyst for oxygen reduction reaction, oxygen and hydrogen evolution reaction. J Colloid Interface Sci 608:2623–2632CrossRef Xu F, Zhao J, Wang J, Guan T, Li K (2022) Strong coordination ability of sulfur with cobalt for facilitating scale-up synthesis of Co9S8 encapsulated S, N co-doped carbon as a trifunctional electrocatalyst for oxygen reduction reaction, oxygen and hydrogen evolution reaction. J Colloid Interface Sci 608:2623–2632CrossRef
Zurück zum Zitat Zang Y, Niu S, Wu Y, Zheng X, Cai J, Ye J, Xie Y, Liu Y, Zhou J, Zhu J, Liu X, Wang G, Qian Y (2019) Tuning orbital orientation endows molybdenum disulfide with exceptional alkaline hydrogen evolution capability. Nat Commun 10:1217CrossRef Zang Y, Niu S, Wu Y, Zheng X, Cai J, Ye J, Xie Y, Liu Y, Zhou J, Zhu J, Liu X, Wang G, Qian Y (2019) Tuning orbital orientation endows molybdenum disulfide with exceptional alkaline hydrogen evolution capability. Nat Commun 10:1217CrossRef
Zurück zum Zitat Zhan G, Yao Y, Quan F, Gu H, Liu X, Zhang L (2022) D-band frontier: a new hydrogen evolution reaction activity descriptor of Pt single-atom catalysts. J Energy Chem 72:203–209CrossRef Zhan G, Yao Y, Quan F, Gu H, Liu X, Zhang L (2022) D-band frontier: a new hydrogen evolution reaction activity descriptor of Pt single-atom catalysts. J Energy Chem 72:203–209CrossRef
Zurück zum Zitat Zhang L, Si R, Liu H, Chen N, Wang Q, Adair K, Wang Z, Chen J, Song Z, Li J (2019) Atomic layer deposited Pt-Ru dual-metal dimers and identifying their active sites for hydrogen evolution reaction. Nat Commun 10:4936CrossRef Zhang L, Si R, Liu H, Chen N, Wang Q, Adair K, Wang Z, Chen J, Song Z, Li J (2019) Atomic layer deposited Pt-Ru dual-metal dimers and identifying their active sites for hydrogen evolution reaction. Nat Commun 10:4936CrossRef
Zurück zum Zitat Zhang J, Zhang L, Liu J, Zhong C, Tu Y, Li P, Du L, Chen S, Cui Z (2022) OH spectator at IrMo intermetallic narrowing activity gap between alkaline and acidic hydrogen evolution reaction. Nat Commun 13:5497CrossRef Zhang J, Zhang L, Liu J, Zhong C, Tu Y, Li P, Du L, Chen S, Cui Z (2022) OH spectator at IrMo intermetallic narrowing activity gap between alkaline and acidic hydrogen evolution reaction. Nat Commun 13:5497CrossRef
Zurück zum Zitat Zhao W, Luo C, Lin Y, Wang G-B, Chen HM, Kuang P, Yu J (2022a) Pt–Ru dimer electrocatalyst with electron redistribution for hydrogen evolution reaction. ACS Catal 12:5540–5548CrossRef Zhao W, Luo C, Lin Y, Wang G-B, Chen HM, Kuang P, Yu J (2022a) Pt–Ru dimer electrocatalyst with electron redistribution for hydrogen evolution reaction. ACS Catal 12:5540–5548CrossRef
Zurück zum Zitat Zhao Y, Kumar PV, Tan X, Lu X, Zhu X, Jiang J, Pan J, Xi S, Yang HY, Ma Z, Wan T, Chu D, Jiang W, Smith SC, Amal R, Han Z, Lu X (2022b) Modulating Pt–O–Pt atomic clusters with isolated cobalt atoms for enhanced hydrogen evolution catalysis. Nat Commun 13:2430CrossRef Zhao Y, Kumar PV, Tan X, Lu X, Zhu X, Jiang J, Pan J, Xi S, Yang HY, Ma Z, Wan T, Chu D, Jiang W, Smith SC, Amal R, Han Z, Lu X (2022b) Modulating Pt–O–Pt atomic clusters with isolated cobalt atoms for enhanced hydrogen evolution catalysis. Nat Commun 13:2430CrossRef
Zurück zum Zitat Zheng Y, Jiao Y, Li LH, Xing T, Chen Y, Jaroniec M, Qiao SZ (2014) Toward design of synergistically active carbon-based catalysts for electrocatalytic hydrogen evolution. ACS Nano 8:5290–5296CrossRef Zheng Y, Jiao Y, Li LH, Xing T, Chen Y, Jaroniec M, Qiao SZ (2014) Toward design of synergistically active carbon-based catalysts for electrocatalytic hydrogen evolution. ACS Nano 8:5290–5296CrossRef
Zurück zum Zitat Zheng J, Sheng W, Zhuang Z, Xu B, Yan Y (2016) Universal dependence of hydrogen oxidation and evolution reaction activity of platinum-group metals on pH and hydrogen binding energy. Sci Adv 2:e1501602CrossRef Zheng J, Sheng W, Zhuang Z, Xu B, Yan Y (2016) Universal dependence of hydrogen oxidation and evolution reaction activity of platinum-group metals on pH and hydrogen binding energy. Sci Adv 2:e1501602CrossRef
Metadaten
Titel
Activity Descriptors for Atomically Precise HER Electrocatalysts
verfasst von
Yasemin Aykut
Ayşe Bayrakçeken Yurtcan
Copyright-Jahr
2024
DOI
https://doi.org/10.1007/978-3-031-54622-8_14